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# Discrete unified gas kinetic scheme for multiscale anisotropic radiative heat transfer

*Advances in Aerodynamics*
**volume 2**, Article number: 3 (2020)

## Abstract

In this work, a discrete unified gas kinetic scheme (DUGKS) is developed for radiative transfer in anisotropic scattering media. The method is an extension of a previous one for isotropic radiation problems [1]. The present scheme is a finite-volume discretization of the anisotropic gray radiation equation, where the anisotropic scattering phase function is approximated by the Legendre polynomial expansion. With the coupling of free transport and scattering processes in the reconstruction of the flux at cell interfaces, the present DUGKS has the nice unified preserving properties such that the cell size is not limited by the photon mean free path even in the optical thick regime. Several one- and two-dimensional numerical tests are conducted to validate the performance of the present DUGKS, and the numerical results demonstrate that the scheme is a reliable method for anisotropic radiative heat transfer problems.

## Introduction

Radiative heat transfer appears in many engineering applications, such as short-pulsed laser in turbid media [2], radiative base heating from rocket exhaust plums [3], radiation in liquid rocket engines [4], nonequilibrium radiative hypersonic flows [5], and some other processes [6–9]. In practical applications, the scattering media are usually anisotropic [10], and some studies have been reported in the literature. For instance, it is found that radiative heat transfer can be greatly influenced in aerosol media due to the anisotropy properties [11]. The physically realistic approach for the scattering behaviour of coal combustion particles is the anisotropic, strongly forward scattering [12]. The liquid aluminum oxide particles produced from combustion of solid propellant exhibit a strong forward scattering characteristic [13].

Radiative heat transfer in anisotropic media can be described by the radiative transfer equation (RTE) for radiation intensity of the photon, which is a high dimensional integral-differential equation. As the scattering effect of the media is strong (optical thick), i.e., the photon mean free path (MFP) *λ* is much smaller than the characteristic macroscopic length *L*, the radiation behaves diffusively. On the other hand, the radiation can transport freely with the light speed when the scattering effect is weak (optical thin). Many practical media contain both strong and weak scattering regimes, such that it is necessary to design numerical schemes which can capture the radiation transport accurately in both cases uniformly. The widely used stochastic Monte Carlo method (MCM) [14–16], which simulates the RTE by tracking the transport process of simulated photons with a mesh size smaller than the MFP, is inefficient in optical thick media. The classical deterministic discrete ordinates method (DOM) [17–19] and finite volume method (FVM) [10, 20–22] also suffer similar challenges. Therefore, it is necessary to develop multiscale schemes which are suitable for problems with arbitrary optical thickness without the limitation of the mesh size by the MFP.

The asymptotic preserving (AP) scheme for the linear kinetic equation is one of the idealized multiscale schemes. AP schemes are first studied in steady neutron transport problems [23–26]. For unsteady problems, some AP schemes have also been proposed [27, 28]. Recently, an AP method, the unified gas kinetic scheme (UGKS) was successfully developed for radiative transfer problems [29–31]. Another asymptotic preserving multiscale method, the discrete unified gas kinetic scheme, which was initially designed for gas flows [32, 33], was also extended to solve the radiative heat transfer problems in isotropic scattering media [1]. As the distribution function at a cell interface in DUGKS is constructed from the characteristic numerical solution rather than the local integral one in the UGKS, the DUGKS has a simpler structure and is more computational efficient. Furthermore, it can be shown that the DUGKS has the unified preserving properties such that it can serve as an efficient multiscale method [34]. However, both the UGKS and DUGKS have not considered the effects of the anisotropic scattering properties.

In present work, we will extend the DUGKS for isotropic radiative transfer to problems with anisotropic scattering effects. With the considering of the anisotropy, the radiative transfer features of the forward scattering media and the backward scattering media can be described clearly. The major difficulty of simulating the anisotropic problem stems from the change of the anisotropic scattering phase function in the RTE. In the present study, the anisotropic phase function will be calculated from the Legendre polynomial expansions [35, 36].

The remainder of this paper is organized as follows. Section 2 introduces the anisotropic scattering radiative transfer equation, and the DUGKS for RTE is described in Section 3. Some numerical tests are performed in Section 4. Finally, a brief summary is given in Section 5.

## Gray radiative transfer equation

The gray radiative transfer equation with anisotropic scattering reads [37, 38]

where *I*(** x**,

**,**

*s**t*) is the distribution function of radiation intensity of photons, related to the spatial position

**, the direction of photon propagation**

*x***and time**

*s**t*.

*c*is the light speed,

*β*is the extinction coefficient which is the inverse of the local photon MFP, i.e.,

*β*=1/

*λ*.

*S*(

**,**

*x***,**

*s**t*) is the source term of the RTE, and

*ω*is the scattering albedo. The function

*I*

_{b}(

**,**

*x**t*) is the blackbody intensity. For equilibrium radiative problems, the blackbody intensity can be calculated according to energy conservation,

where *Ω* is the solid angle domain of ** s**. For radiative nonequilibrium problems, when the temperature field of the medium is given, the blackbody intensity can be calculated by the Stefan-Boltzmann law [37], i.e.,

where *σ* is the Stefan-Boltzmann constant and *T* is the local temperature of the medium, and *Φ*(*s*^{′},** s**) is the scattering phase function, which describes the fraction of the radiative energy scattered into the outgoing direction

**from the incoming direction**

*s*

*s*^{′}, and

*Ω*

^{′}is the corresponding solid angle domain. In the RTE, the anisotropic scattering characteristic of the participating media is fully expressed by the scattering phase function

*Φ*(

*s*^{′},

**), which satisfies the normalization condition,**

*s*Unlike the isotropic scattering problems where the scattering phase function is constant (*Φ*≡1), the scattering phase function in anisotropic scattering problems changes according to the scattering angle. In this study it is approximated by a finite series of Legendre polynomials [17, 35, 36], i.e.,

where *ψ* is the angle between incoming direction *s*^{′}(*μ*^{′},*φ*^{′}) and scattered direction ** s**(

*μ*,

*φ*).

*μ*is the cosine of the zenith angle and

*φ*is the azimuth angle of the direction

*s*.

*C*

_{j}(

*α*

_{1},

*α*

_{2}) is the angular distribution coefficients, where

*α*

_{1}=

*π*

*D*/

*υ*and

*α*

_{2}=

*m*

*π*

*D*/

*υ*with

*D*being the diameter of radiative medium particle,

*υ*is the wavelength of the incident radiation in the surrounding medium, and

*m*is the complex index of refraction of radiative medium particle relative to the surrounding medium.

*P*

_{j}is Legendre polynomials of order

*j*. For strongly anisotropic scattering media, the upper limit

*N*should be big enough to ensure the accuracy of the calculation results.

In radiative transfer, the incident radiation energy *G* and heat flux *q* are two important physical quantities, which are defined from the radiation intensity,

## Numerical scheme

### DUGKS with anisotropic scattering effects

In this section, the discrete unified gas kinetic scheme for gray radiative transfer equation involving the anisotropic scattering effects (Eq. (1)) is constructed in detail. Similar to the discretization approach in Ref [39], the solid angle space is discretized into *M* discrete angles using the discrete ordinates method based on certain spherical quadratures, and correspondingly we obtain *M* discrete directions *s*_{k}. With these discrete directions, the RTE (1) can be expressed as

where *k*,*m*=1,2,...,*M*, and *ω*_{m} is the weight assigned to the discretized direction *s*_{m}. Following Refs. [1, 32], integrating Eq. (10) on a control volume *V*_{j} centered at *x*_{j} from time *t*_{n} to *t*_{n+1}=*t*_{n}+△*t*, we can obtain

where

is the flux across the cell interface, *I*(*x*_{j},*s*_{k},*t*_{n}) denotes the cell averaged value for the diffuse intensity at time *t*_{n} with control volume of *V*_{j} located at *x*_{j} along photon propagation direction *s*_{k}, *n*_{f} is the outward unit normal vector at *x*_{f} of an interface, and △*S*_{f} is the corresponding interface area. The midpoint rule for the integration of the second term on the left-hand of Eq. (12) and trapezoidal rule for the right-hand of Eq. (12) are used, respectively. Two new distribution functions are introduced to remove the implicitness in Eq. (12),

where *χ*=*c**β*△*t*. Then Eq. (12) can be rewritten as

In order to evaluate the cell interface flux at the half time-step *F*^{n+1/2}, we integrate Eq. (10) along the characteristic line with a half time step,

where *h*=△*t*/2, and the trapezoidal rule is again used to evaluate the right-hand term of Eq. (10). Another two new distribution functions are also introduced to remove the implicitness in Eq. (17),

Substituting Eqs. (18) and (19) into Eq. (17), we can obtain

\(\bar {I}^{+} \left (\boldsymbol {x}_{f} - \boldsymbol {s}_{k} c h, \boldsymbol {s}_{k}, t_{n} \right)\) can be reconstructed by

where **σ**_{j} is the slope of the distribution function \({\bar {I}}^{+} \) in cell *j*. In the present study, the van Leer limiter [40] is used to calculate the slope.

The new distribution functions \(\widetilde {I}, {\widetilde {I}}^{+}, \bar {I}, {\bar {I}}^{+}\) are all related to the original distribution function *I* and the scattering phase function *Φ*(*c**o**s**ψ*). Their relations in the present work can be finally obtained as

In the isotropic scattering condition (*Φ*≡1), Eqs. (22) and (23) can be solved explicitly [1]. However, in anisotropic case, due to the complexity of the phase function (*Φ*(*s*^{′},** s**)), Eqs. (22) and (23) can not be solved explicitly. Here a simple iterative method is employed as follows. First, the iteration procedure for the calculation of the original distribution function

*I*(

*x*_{f},

*s*_{k},

*t*

_{n+1/2}) is

where *l* is the iteration index, and

The iteration stops as the intensity is converged, i.e., ∣*I*^{l+1}−*I*^{l}∣<*ε*, where *ε* is a small number which is set to be 10^{−4} in our simulations. Eq. (23) is also solved iteratively in a similar way. We found that the number of iterations is less than 10 in almost all the numerical tests in the present work. But for more complex problems, more advanced acceleration technique should be employed.

Finally, we note that with the use of the trapezoidal rule in Eqs. (12) and (17), the present DUGKS is a semi-implicit scheme and the time step *Δ**t* is not limited by the scattering, which is determined by the Courant-Friedrichs-Lewy (CFL) condition [41],

where 0<*α*<1 is the CFL number, and *Δ**x* is the minimal grid spacing.

### Boundary conditions

In the present work, diffusely emitting and reflecting boundaries are considered. When the wall is black, a photon is absorbed as it hits the wall, and a new photon in thermal equilibrium with boundary temperature is emitted into the domain. When the wall is gray, some of the incident photons are absorbed and the rest are reflected diffusively back to the domain, depending on the reflectivity of the wall. The general boundary condition for Eq. (1) can be expressed as

where *ε*_{w} is the diffuse emissivity, *ρ*_{w} is the diffuse reflectivity, and *n*_{w} is the unit inner normal vector at the boundary. *I*_{b}(*x*_{w}) is the blackbody radiation intensity at the boundary surface having a specified temperature. This boundary condition is implemented in the DUGKS straightforwardly by replacing the *s* with each discrete angle *s*_{k}, and evaluating the integral with the numerical quadrature.

### Algorithm

In summary, the main procedure of the DUGKS from time step *t*_{n} to *t*_{n+1} can be summarized as follows:

- 1.
Calculate the microflux

*F*^{n+1/2}at cell interface*x*_{f}and at time*t*_{n+1/2}.- (a)
Calculate \({\bar {I}}^{+}\) from \(\widetilde {I}\) at each cell center with the iterative method according to Eq. (23);

- (b)
Reconstruct the slope

**σ**_{j}of \({\bar {I}}^{+}\) in each cell center; - (c)
Reconstruct the distribution function \({\bar {I}}^{+}\) at

*x*_{f}−*s*_{k}*c**h*according to Eq. (21); - (d)
Calculate the distribution function \(\bar {I}\) at cell interface at time

*t*_{n+1/2}according to Eq. (20); - (e)
Calculate the original distribution function

*I*at cell interface and at time*t*_{n+1/2}with the iterative method according to Eq. (25); - (f)
Calculate the microflux

*F*^{n+1/2}through each cell interface from*I*(*x*_{f},*s*_{k},*t*_{n+1/2}) according to Eq. (13).

- (a)
- 2.
Calculate \({\widetilde {I}}^{+} \) at cell center and at time

*t*_{n}according to Eq. (24). - 3.
Update the cell averaged \(\widetilde {I}\) in each cell from

*t*_{n}to*t*_{n+1}according to Eq. (16).

When the transformed intensity distribution is known, the local incident radiation energy can be calculated based on Eq. (14)

and the net radiative heat flux can be calculated based on Eqs. (14) and (19),

## Numerical examples

In this section, three radiative transfer problems in anisotropic scattering media are simulated to validate the proposed DUGKS, including the radiative transfer in a slab with different wall temperatures, radiative transfer in a square domain with a hot wall, and radiative transfer in a square domain with collimated incidence. In each case, Cartesian coordinates is used to discretize the physical space, and the Gauss-Legendre quadrature [42] is used for angular discretization, where *μ*∈[−1,1] and *φ*∈[0,2*π*] are the cosine of zenith and azimuth angle, respectively. The CFL number is taken to be *α*=0.5. For steady problems, the system is regarded as converged as *E*<10^{−6}, where

### Radiation in a slab with different wall temperatures

In the first case, the DUGKS is applied to the radiative heat transfer in a slab with thickness *L* filled with anisotropic absorbing-scattering media, as shown in Fig. 1. The temperatures on the boundaries located at *x*=0 and *x*=*L* are maintained at *T*_{0} and *T*_{1}, respectively, where *T*_{1}>*T*_{0}. The angular space is discretized into 40 control angles. The physical space is discretized into *N*_{x}=21 uniform cells. Two anisotropic media composed of different particle clouds are considered, where the radiative properties are summarized in Table 1. The scattering phase function is expressed by *N*-th Legendre polynomial expansions obtained from Eq. (6). Figure 2 shows the non-dimensional radiation energy *Φ*_{b} at different optical thickness *τ*=*β**L*, where *Φ*_{b}=(*G*−*G*_{0})/(*G*_{1}−*G*_{0}) with \(G_{0} = 4\sigma T^{4}_{0}\) and \(G_{1} = 4\sigma T^{4}_{1}\). It can be seen that the results are in good agreement with the exact results for *τ*=0.1,1,5 [43]. When *τ* is large, the incident radiation energy *G* can be solved by the limit diffusion equation such that the distribution of *G* is linear, where the optical thick cases for *τ*=21,40,100,1000 agree well with that. It is noted that the results are still satisfied even as *Δ**x*/*λ*=*τ*/*N*_{x}≥1. These results confirm the capability of the present DUGKS method in simulating anisotropic heat transfer process for one-dimensional problems.

### Radiation in a square domain with a hot wall

In this subsection, we consider a square with the side length of *L* enclosed by four boundaries, as shown in Fig. 3. The bottom wall is kept hot with a non-dimensional temperature of *T*_{1}=1, while the other walls and the media are kept cold with a non-dimensional temperature of *T*_{0}=0.

A grid size of *N*_{x}×*N*_{y}=26×26 is used for physical space discretization. The direction cosine of zenith angle *μ*∈[−1,1] is discretized with *N*_{μ}=16 points, while the azimuth angle *φ*∈[0,2*π*] is discretized into *N*_{φ}=16 points. The scattering albedo is set to be *ω*=1.0. Four different kinds of anisotropic scattering media and the isotropic scattering medium are considered. Table 2 shows the expansion coefficients *C*_{j} and the asymmetry factors *C*_{j}/3 of the phase function for different scattering media [17]. The anisotropic and isotropic scattering phase functions varying with the scattering angle are shown in Fig. 4. It can be observed that the phase function for the anisotropic scattering media changes dramatically with the change of the scattering angle, which will significantly influence the energy transfer in practical problems.

Figure 5 shows the net radiative heat flux in the *y*-direction along the vertical centerline at *x*=*L*/2. The net hot surface radiative heat flux is shown in Fig. 6. For comparison, we also present the solutions of DOM [17] for this problem. It can be seen the DUGKS results agree quite well with the DOM results for five different media. From Fig. 5 and Fig. 6, the effects of the anisotropic scattering media can be seen clearly. The forward scattering media transport more radiation heat into the forward direction than the isotropic medium, while the backward scattering media transport less radiation heat into the forward direction than the isotropic medium.

The effect of the wall reflectivity on the radiative heat transfer is also examined with the medium *F*2. Figure 7 shows the net radiative heat flux along the centerline of the enclosure at different wall reflectivity. It is noted that with the increasing of *ρ*, the radiative heat flux *q*_{y} decreases significantly, which is caused by the increasing of the radiative flux that reflects from the walls.

The net radiative heat flux along the centerline *q*_{y} for different optical thickness with the medium *F*2 is also shown in Fig. 8. The optical thickness range from *τ*=0.01 to *τ*=100 are considered. The DUGKS results agree well with the DOM results [17] from *τ*=0.01 to *τ*=10, and have the reasonable results when *Δ**x*/*λ*=*τ*/*N*_{y}≥1. Furthermore, in the literature [17], when the optical thickness is larger than 2.5, the DOM scheme should use finer mesh (52×52) to eliminate the error. The DUGKS does not have this problem, as shown in Fig. 8. These results again confirm the capability of the present DUGKS method in simulating 2D anisotropic radiative scattering problems.

### Radiation in a square domain with collimated incidence

To further test the capability of the present DUGKS method in simulating radiative transfer problem with anisotropic scattering media, we now apply it to 2D square problems with collimated incidence. As shown in Fig. 9, the side length of the square is *L*. All walls and the interior domain are kept cold with the temperature *T*_{0}. A collimate beam (*I*_{c}=*π*) is incident through the top boundary. The collimate beam is normal to the top boundary.

The discretization of the physical space is *N*_{x}×*N*_{y}=26×26. The solid angle is discretized with *N*_{μ}×*N*_{φ}=16×16. The scattering albedo is taken to be *ω*=1.0. The parameters of phase function for anisotropic scattering media are shown in Table 2. In this test, with the collimated incidence from the top wall the radiative transfer equation now can be expressed as follows [18],

where *s*_{c} is incident angle of the beam, and *τ*_{y}=*β**y*.

The walls energy losses for the different phase functions are illustrated in Fig. 10. Fig. 10a shows the reflected components of the radiative flux along the top wall, and the transmitted components of the radiative flux along the bottom wall are shown in Fig. 10b. It is observed that the DUGKS results agree well with the DOM results [18] in all cases. From these figures, the same conclusions as in section 4.2 that backward scattering media reflect more radiative energy while forward scattering media transmit more energy can also be obtained. The side walls energy losses for the different phase functions are shown in Fig. 10c.

The net radiative heat flux along the centerline *q*_{y} for different anisotropic scattering media and different optical thickness are shown in Fig. 11 and Fig. 12, respectively. All of them agree well with the DOM solutions [18]. These tests clearly show that the DUGKS is an accurate solver for radiative transfer with anisotropic scattering media.

## Summary

In present work, we developed a discrete unified gas kinetic scheme for radiative transfer with anisotropic scattering media based on the radiative transfer equation. Due to the complex anisotropic scattering phase function which is calculated by the Legendre polynomial expansion, a simple and efficient iterative approach is employed. The present DUGKS has been validated by a set of radiative transport problems including the radiative transfer in a slab with different wall temperatures, radiative transfer in a square domain with a hot wall, and radiative transfer in a square domain with collimated incidence. All results agree well with other different numerical schemes. In these cases, even if the mesh size is larger than the photon mean free path, the results predicted by the present scheme are still reliable. As the scheme has the nice unified preserving properties and the mesh size is not restricted by the photon mean free path, the present DUGKS will be an efficient and accurate tool to describe the multiscale anisotropic radiative heat transfer. It will also be easy to handle more complex radiative transfer problems with unstructured meshes, due to its finite volume property.

## Availability of data and materials

All data generated or analyzed during this study are included in this published article.

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## Acknowledgments

This work was supported by the National Key R&D Program of China (No. 2018YFE0180900) and the Fundamental Research Funds for the Central Universities (No. 2019kfyXMBZ040).

## Funding

The National Key R&D Program of China (No. 2018YFE0180900) and the Fundamental Research Funds for the Central Universities (No. 2019kfyXMBZ040).

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Song, X., Zhang, C., Zhou, X. *et al.* Discrete unified gas kinetic scheme for multiscale anisotropic radiative heat transfer.
*Adv. Aerodyn.* **2, **3 (2020). https://doi.org/10.1186/s42774-019-0026-3

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DOI: https://doi.org/10.1186/s42774-019-0026-3

### Keywords

- Gray radiative transfer equation
- Anisotropic scattering
- Scattering phase function
- Legendre polynomial